Fabrication and near-infrared optical responses of 2D periodical Au/ITO nanocomposite arrays

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摘要 Two-dimensional(2D)periodicalAuandindiumtinoxide(ITO)nanocompositearrayshavebeenfabricatedbasedonaself-assemblednanospherelithographytechnique.Abutton-shapedAunanoparticlewasformedoneachhollowhemisphere-shapedITOshell.Importantly,theunderlyingformationmechanismduringthethermaltreatmenthasbeenthoroughlyexploredbycomparingstructuresresultingfromdifferentdepositionconditionsindetail.ComparedtotheAunanoparticlearrayswithoutITOshells,theAu/ITOnanocompositearraysshowedastrongerlocalizedsurfaceplasmonresonanceeffectandhigherabsorptioninthenear-infrared(NIR)region,benefitingfromthefree-electroninteractionenhancementbetweenAuandITO.Thenonlinearopticalpropertieswereinvestigatedusingamodifiedfemtosecondintensity-scansystem,andtheresultsdemonstratedAu/ITOnanocompositearrayswitharemarkabletwo-photonabsorptionsaturationeffectforfemtosecondpulsesat1030nm.TheversatileNIRopticalresponsesindicatethegreatpotentialoftheelaboratelyprepared2DperiodicalAu/ITOnanocompositearraysinmanyapplicationssuchassolarcells,photocatalysis,andnovelnanooptoelectronicdevices.
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出版日期 2017年04月14日(中国Betway体育网页登陆平台首次上网日期,不代表论文的发表时间)
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